using (PdfDocument one = PdfReader.Open("file1.pdf", PdfDocumentOpenMode.Import))
using (PdfDocument two = PdfReader.Open("file2.pdf", PdfDocumentOpenMode.Import))
using (PdfDocument outPdf = new PdfDocument())
{                
    CopyPages(one, outPdf);
    CopyPages(two, outPdf);

    outPdf.Save("file1and2.pdf");
}

void CopyPages(PdfDocument from, PdfDocument to)
{
    for (int i = 0; i < from.PageCount; i++)
    {
        to.AddPage(from.Pages[i]);
    }
}